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Journal of Sustainable Cement-Based Materials· 2026Q1

Heterojen çimentolu atık ince tanelerinin zorlanmış sulu karbonatasyonu: CO 2 alımı ve Portland çimentosunda katkı çimento malzemeleri olarak performansı

Enforced aqueous carbonation of heterogeneous cementitious waste fines: CO 2 uptake and performance as supplementary cementitious materials in Portland cement

Mateus Zanovello, Sérgio C. Angulo

Kısa özet

Çimentolu atıkların zorlanmış sulu karbonatasyonu, çimentolu sertleşmiş macun, beton yıkama çamuru ve genç CDW ince taneleri gibi malzemelerde yüksek CO2 alımı (%372 kg CO2/t'ye kadar) sağlamış ve Portland çimentosunda mukavemeti %27-34 (7 gün) ve %40-45 (28 gün) artıran katkı çimento malzemeleri (SCM'ler) üretmiştir.

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Özet (abstract)

Enforced carbonation of cementitious wastes is a strategy to mitigate CO2 emissions and generate reactive supplementary cementitious materials (SCMs), yet few studies have analyzed real sources. In this study, three heterogeneous wastes were investigated: hardened cement paste (HCP), concrete truck washout sludge (RCS), and young CDW fines (YCW). The hydrated cement content of the cementitious wastes was 87%, 62%, and 28%, respectively. Enforced aqueous carbonation (100% CO2, 0.02 L·min−1·g−1, L/S 10:1, 6 h) was applied. Carbonation degrees reached 99%, 76%, and 88%, while CO2 uptake was 372, 112, and 69 kg CO2/t. Specific surface area increased up to 156%, and mesoporosity doubled. Carbonated powders tested as SCMs at 30% clinker replacement delivered 27–34% strength gains at 7 days and 40–45% at 28 days above dilution, with RCS matching HCP performance. Carbonation degree alone was insufficient to assess carbonation performance; quantity of CaO available governs both sequestration efficiency and SCM quality.

Yazarların özeti; kaynağından alınmıştır. Journal of Sustainable Cement-Based Materials, 2026 · DOI ↗

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