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Scientific Reports· 2026Q1

Advanced experimental analysis on the synthesis and modification of zinc iron-based nanoparticles for separation and removal of pharmaceutical compounds

Sawsan B. Eltahir, Kamal Y. Thajudeen, Mohammed Muqtader Ahmed, Saad Ali Alshehri

Short summary

Porous Co-doped ZnFe₂O₄ microspheres (15% Co-ZF) achieved 93% tetracycline (TC) degradation under visible light, showing potential for water purification.

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Key points

  • Porous Co-doped ZnFe₂O₄ microspheres were synthesized and tested for tetracycline (TC) degradation.
  • The 15% Co-ZF catalyst achieved 93% TC degradation under visible light at 20 mg/L catalyst loading, pH 5.52, and 100 W LED lamp after 240 min.
  • Catalyst reusability showed a 9% efficiency decrease over three cycles, indicating good stability.
  • ·OH radicals were identified as the primary reactive species responsible for degradation.

AI-generated from the title and abstract; the full text is not read.

Abstract

This study reports the visible-light-driven photocatalytic degradation of tetracycline (TC) in aqueous media using porous Co-doped ZnFe₂O₄ microspheres. ZnFe 2 O 4 (ZF) microspheres with a porous, spherical morphology were synthesized and subsequently doped with 5 wt% and 15 wt% cobalt (Co). The produced photocatalysts were subsequently assessed for their TC degradation performance under visible light irradiation from an LED lamp. The 15% Co-ZF catalyst showed the highest degradation efficiency among the three catalytic materials. A systematic study was conducted to assess the influence of TC concentration, catalyst concentration, pH, and lamp intensity on degradation efficiency. A degradation percentage of 92% was observed with a catalyst loading of 20 mg/L and the lowest TC concentration. Optimal degradation of 93% was achieved for 15%Co-ZF under 100 W LED lamp at pH = 5.52 after 240 min. Reusability studies revealed a slight decrease in degradation efficiency over three cycles, with a 9% reduction in the third cycle, indicating acceptable stability of the sample. Post-reaction XRD/FTIR analyses confirmed the structural stability of the photocatalyst, while scavenger experiments identified ·OH radicals as the dominant reactive species. These results highlight the potential of Co-doped ZF microspheres as efficient and reusable photocatalysts for the removal of TC from contaminated water sources.

The authors' abstract, as published at the source. Scientific Reports, 2026 · DOI ↗

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Field: Renewable Energy, Sustainability and the Environment

Renewable Energy, Sustainability and the EnvironmentEnergy